I've attended anime conventions and given writing panels since 2012, and one of my favorite things to do (although it's not always easy to) is meet voice actors for some of my favorite series!
I've had the pleasure of meeting several VAs you'd recognize (most of them through Funimation productions), and when I'm not overly starstruck (unfortunately this does happen), I try to ask each VA the exact same question:
What is something you're really proud of that you'd like me to see?
I ask this because there's still a lot of anime I'm not familiar with (but I am definitely catching up!), and also because I wonder if there are other roles each actor has played that might be overlooked because they weren't star-makers or fan favorites.
It's also easy to forget that a lot of VAs perform roles outside of acting when it comes to localizing anime, such as scriptwriting, ADR, and directing; this is another reason why I thought I'd give the actor the opportunity to recommend me a show based on their personal feelings about it.
I've been hit-and-miss with my interactions with VAs (I get irrationally nervous around them), so unfortunately my ratio of answers to actors is grievously slim. I hope to continue to build this list over time.
In the meantime, I have the VA name hyperlinked to their bio/cast lists, their response to me in bold, and the plot synopsis of the series, which is sourced from MyAnimeList.net (because I haven't watched most of these yet). Enjoy!
Black Lagoon - "Okajima Rokuro is a Japanese businessman in a town full of Japanese businessmen. His normal day consists of social drinking with clients and being kicked around by his bosses. He finally gets a break though, as he's sent by his company to the tropical seas of Eastern China to deliver a disc. But his boat gets hijacked by a band of mercenaries hired to retrieve the disc. Rock (as he is newly dubbed by his captors) catches the interest of the only female merc Revy as she thinks he's worth a ransom, taking him hostage. However, the disc that was stolen has a terrible secret that's unknown to Rock, which causes massive confusion and chaos for both him and his kidnappers."
Baccano! - "During the early 1930s in Chicago, the transcontinental train, Flying Pussyfoot, is starting its legendary journey that will leave a trail of blood all over the country. At the same time in New York, the ambitious scientist Szilard and his unwilling aide Ennis, are looking for missing bottles of the immortality elixir. In addition, a war between the mafia groups is getting worse. On board the Advena Avis, in 1711, alchemists are about to learn the price of immortality.
Based on the award winning light novels of the same name, this anime adaptation follows several events that initially seem unrelated, both in time and place, but are part of a much bigger story—one of alchemy, survival and immortality. Merging these events together are the kindhearted would-be thieves, Isaac and Miria, connecting various people, all of them with their own hidden ambitions and agendas, and creating lifelong bonds and consequences for everyone involved."
Wolf's Rain - "In some distant future, it's common knowledge that all wolves have been extinct for 200 years. However, it seems this is false as wolves have not disappeared but rather have taken human form. Kiba, a lone wolf, wanders into a city, trying to sniff out the Lunar Flowers that are supposed to lead whoever follows the scent to paradise. The source of the smell is Cheza, a girl who sleeps in what appears to be suspended animation in a lab. She and the wolves are drawn to each other, and Kiba hopes to find paradise once he finds the source of the scent of Lunar Flowers. However, once Kiba finds Cheza, she is kidnapped by a mysterious person called Darcia, and his search begins anew. Before he leaves the city, he meets 3 other wolves, Tsume, Hige and Toboe. All four wolves have very different personalities and ideas, and their friendliness towards each other is a little rough around the edges. However, they soon band together to continue to search for paradise."
Code Geass - "On August 10th of the year 2010 the Holy Empire of Britannia began a campaign of conquest, its sights set on Japan. Operations were completed in one month thanks to Britannia's deployment of new mobile humanoid armor vehicles dubbed Knightmare Frames. Japan's rights and identity were stripped away, the once proud nation now referred to as Area 11. Its citizens, Elevens, are forced to scratch out a living while the Britannian aristocracy lives comfortably within their settlements. Pockets of resistance appear throughout Area 11, working towards independence for Japan.
Lelouch, an exiled Imperial Prince of Britannia posing as a student, finds himself in the heart of the ongoing conflict for the island nation. Through a chance meeting with a mysterious girl named C.C., Lelouch gains his Geass, the power of the king. Now endowed with absolute dominance over any person, Lelouch may finally realize his goal of bringing down Britannia from within!"
Eden of the East - "On November 22, 2010 ten missiles strike Japan. However, this unprecedented terrorist act, later to be known as "Careless Monday," does not result in any apparent victims, and is soon forgotten by almost everyone. Then, 3 months later... Saki Morimi is a young woman currently in the United States of America on her graduation trip. But just when she is in front of the White House, Washington DC, she gets into trouble, and only the unexpected intervention of one of her fellow countrymen saves her. However, this man, who introduces himself as Akira Takizawa, is a complete mystery. He appears to have lost his memory, is stark naked, except for the gun he holds in one hand, and the mobile phone he's holding in the other. A phone that is charged with 8,200,000,000 yen in digital cash."
Ouran High School Host Club - "Fujioka Haruhi wins a scholarship to attend Ouran Academy, a school reserved for only the most rich and prestigious. Despite what other students may think of her, she cares little for physical appearances or the fact that she is a commoner.
Unfortunately for Haruhi, her high school days take a sudden turn when she stumbles upon the Host Club, an elite club filled with super rich and beautiful boys who use their specific traits and charms to entertain young ladies. Even worse, Haruhi accidentally breaks an 8-million yen vase in the club. Since she is unable to repay her debt with money, Haruhi finds herself with no choice but to work for the Host Club, becoming a male host herself."